Gradient-based optimization of nuclear criticality experiments using neural surrogate eigenvalue sensitivities

arXiv:2606.04033v2 Announce Type: replace Abstract: The validation of advanced nuclear reactor designs and fuel concepts will require the design of new critical experiments with high neutronic similarity to the target technology. Neutronic similarity can be quantified by the correlation coefficient $c_k$, which captures the shared bias in $k_\text{eff}$ induced by uncertainties in nuclear data. Generally, a $c_k\geq0.9$ is needed for an experiment to be sufficiently similar to a target technology. In this work, a physics-informed deep neural network is trained to predict the neutronic sensitivity of grid-based critical experiment geometries. The differentiability of the neural network is used to enable gradient-based design optimization of new experiment geometries to maximize $c_k$ with the sensitivity profile of a target technology. This approach allows for optimization over the combinatorial design space of potential material combinations within the grid, moving beyond traditional parametric optimization approaches. The method is applied to the validation of the TN-Americas TN-LC transportation cask with HALEU fuel, for which existing critical experiment coverage is limited. This application is shown to produce experiment geometries achieving $c_k$ scores of 0.97757, 0.81324, and 0.93276 for three configurations of interest.